The fonds consists of the diaries of Harriet Pengelley (1835-1836), Robert Pengelley (1835), and A.E. Marguerite (Rita) Pengelley (1940-1941); correspondence; sketchbooks (1829-1830); drawings; and photographs. In 1994, an addition was made to the fonds which included a photocopy of a diary of Robert Pengelley (1837-1840) and textual records regarding the Pengelley family. In 2018, an addition of Pengelley family genealogical information was received.